From Bytes to Ingots: Expedient Design of Structural Materials for Advanced Nuclear Energy Systems
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		    1043-T01-01
 
 From Bytes to Ingots: Expedient Design of Structural Materials for Advanced Nuclear Energy Systems Steve Zinkle, Ron Klueh, Phil Maziasz, Jeremy Busby, David Hoelzer, John Vitek, Roger Stoller and Yuri Osetsky © 2008 Materials Research Society Oak Ridge National Laboratory, Oak Ridge, TN
 
 Materials Research Society Fall Meeting Symposium T: Materials innovations for next generation nuclear energy Boston, MA, November 26-30, 2007 OAK RIDGE NATIONAL LABORATORY U. S. DEPARTMENT OF ENERGY
 
 Outline • Brief history of nuclear power • Effects of neutron bombardment on structural materials − “Five scourges” of radiation
 
 • Prospects development of high-performance © 2008for Materials Research Society radiation-resistant materials − Crucial role of nanoscale architectures
 
 OAK RIDGE NATIONAL LABORATORY U. S. DEPARTMENT OF ENERGY
 
 The Launching of Nuclear Energy Largely Preceded the Development of Modern Materials Science
 
 CP-1
 
 Graphite Shippingport reactor EBR-I
 
 TMI
 
 Kyoto protocol
 
 © 2008 Materials Research Society 1940
 
 1950
 
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 Development of Mat. Sci. 1 Tflops as an academic 1 Gflops achieved; discipline Development of high performance Fracture mechanics computing centers established
 
 2010 1 Pflops
 
 •Fusion and Gen IV fission energy systems should take maximum advantage of current and emerging materials and computational science tools OAK RIDGE NATIONAL LABORATORY U. S. DEPARTMENT OF ENERGY
 
 • Radiation hardening and embrittlement (0.1 dpa)
 
 Engineering Stress, MPa
 
 Radiation Damage can Produce Large Changes in Structural Materials USJF82Hss2
 
 1200
 
 Tirr=Ttest
 
 200°C/10 dpa 250°C/3 dpa
 
 1000
 
 400°C/10 dpa
 
 300°C/8 dpa
 
 800
 
 400°C/34 dpa 500°C/34 dpa
 
 600 Unirradiated YS
 
 400 200 0
 
 600°C/ 8 dpa
 
 500°C/8 dpa
 
 0
 
 0.05
 
 0.1
 
 0.15
 
 0.2
 
 0.25
 
 0.3
 
 0.35
 
 Engineering Strain, mm/mm
 
 • Phase instabilities from radiation-induced precipitation (0.3-0.6 TM, >10 dpa)
 
 50 nm
 
 © 2008 Materials • Irradiation creep (10Research dpa)
 
 Society
 
 • Volumetric swelling from void formation (0.3-0.6 TM, >10 dpa) 100 nm
 
 • High temperature He embrittlement (>0.5 TM, >10 dpa) after S.J. Zinkle, Phys. Plasmas 12 (2005) 058101
 
 100 nm
 
 Advanced nuclear energy systems impose harsh radiation damage conditions on structural materials • 1 displacement per atom (dpa) corresponds to stable displacement from their lattice site of all atoms in the material during irradiation near absolute zero (no thermally-activated point defect diffusion) − Initial number of atoms knocked off their lattice site during fast reactor neutron irradiation is ~100 times the dpa value • Most of these originally displaced atoms hop onto another lattice site during “thermal spike” phase of the displacement cascade (~1 ps)
 
 © 2008 Materials Research Society
 
 R.E. Stoller
 
 • Requirement for structural materials in advanced nuclear energy systems (~100 dpa exposure): − ~99.95% of “stable” displacement damage must recombine • ~99.9995% of initially dislodged atoms must recombine
 
 • Two general strategies for radiation resistance can be en		
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