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Editorial Board: A.]. Bard" I.G. Dance" P. Day-].A. Ibers- T. Kunitake T.]. Meyer" D.M.P. Mingos" H.W. Roesky ].-P. Sauvage. A. Simon" F. Wudl

Springer

Berlin Heidelberg New York Barcelona Hong Kong London Milan Paris Singapore Tokyo

Localized to Itinerant Electronic Transition in Perovskite Oxides

VolumeEditor:J.B.Goodenough With contributions by S.L. Cooper, T. Egami, J.B. Goodenough, ].-S. Zhou

~ Springer

The series Structure and Bonding publishes critical reviews on topics of research concerned with chemical structure and bonding. The scope of the series spans the entire Periodic Table. It focuses attention on new and developing areas of modern structural and theoretical chemistry such as nanostructures, molecular electronics, designed molecular solids, surfaces, metal clusters and supramolecular structures. Physical and spectroscopic techniques used to determine, examine and model structures fall within the purview of Structure and Bonding to the extent that the focus is on the scientific results obtained and not on specialist information concerning the techniques themselves. Issues associated with the development of bonding models and generalizations that illuminate the reactivity pathways and rates of chemical processes are also relevant. As a rule, contributions are specially commissioned. The editors and publishers will, however, always be pleased to receive suggestions and supplementary information. Papers are accepted for Structure and Bonding in English. In references Structure and Bonding is abbreviated Struct. Bond. and is cited as a journal. Springer w w w home page: http://www.springer.de

ISSN 0081-5993 ISBN 3-540-67522-1 Springer-Verlag

Berlin Heidelberg New York

CIP Data applied for This work is subject to copyright. All rights are reserved, whether the whole or part of the material is concerned, specifically the rights of translation, reprinting, reuse of illustrations, recitation, broadcasting, reproduction on microfilm or in any other way, and storage in data banks. Duplication of this publication or parts thereof is permitted only under the provisions of the German Copyright Law of September 9, 1965, in its current version, and permission for use must always be obtained from Springer-Verlag. Violations are liable for prosecution under the German Copyright Law. Springer-Verlag Berlin Heidelberg New York a member of BertelsmannSpringer Science + Business Media GmbH © Springer-Verlag Berlin Heidelberg 2001 Printed in Germany The use of registered names, trademarks, etc. in this publication does not imply, even in the absence of a specific statement, that such names are exempt from the relevant protective laws and regulations and therefore free for general use. Typesetting: Scientific Publishing Services (P) Ltd, Madras Production editor: Christiane Messerschmidt, Rheinau Cover: Medio V. Leins, Berlin Printed on acid-free paper SPIN: 10676188 02/3020 - 5 4 3 2 1 0

Volume Editor P r o f e s s o r Dr. J o h n B. G o o d e n o u g h Texas Materials Institute University of Texas at Austi