Magnetoresistance in Granular Metals

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MAGNETORESISTANCE

IN GRANULAR METALS

W.L. MCLEAN Rutgers University, Serin Physics Laboratory, Piscataway,

P.O. Box 849,

NJ 08855

ABSTRACT

We review the origins of the magnetoresistance in

granular metals with

emphasis on the quantum coherence effects arising from the interference electrons

traveling by different

paths.

magnetoresistance expected from scaling arguments and observed in aluminum.

Two theories of the magnetoresistance

hopping regime,

of

We discuss the maximum in the

one based on the magnetic-field

in

granular

the variable range

induced shift

mobility edge and the other dealing with "directed" hopping,

of the

are compared

with experiments.

INTRODUCTION

Granular metals, a rich

variety

complexity. follows its contact,

as this week-long Symposium well demonstrates,

of properties This is

many of which themselves

exhibit

reveal great

certainly true of the magnetoresistance

when one

evolution from the metallic case where the grains are in close

then through the metal-insulation transition,

and finally on into

the hopping conduction regime where the grains are well separated. magnetoresistance in granular metals can be large and negative

(Ap/p

The - -1)

even though experience with impure simple metals might lead us to expect it to be small and positive.

The most obvious anticipated effect of a magnetic

field on an individual grain is

shrinkage of its

electron wavefunctions

which reduces overlap with neighboring grains and hence would also increase the resistance of the system. magnetoresistance,

particularly in

began with the work in

the late

However,

a proper understanding of the

the metallic regime of a granular system, 1970's

and early

localization in metals with increasing disorder localization in

(1].

1980's on the onset of The scaling theory of

particular [2] seemed of such wide generality that it

be directly applicable in

should

the case where the scale of the granularity was

smaller than the relevant length scales of the theory, scattering length or the "magnetic length",

LH,

where

such as the inelastic 2 LH = (tc/eH) [3]. As

Mat. Res. Soc. Symp. Proc. Vol. 195. 11990 Materials Research Society

118

the granular metal is grains,

made more disordered by reducing the concentration of

percolataion

After percolation

effects begin to affect the transport ceases,

electrical

electrons between disconnected concentrations

there is

the magnetoresistance

in

properties.

conduction occurs by hopping of

clusters

of grains.

At still

hopping from grain to grain.

smaller

Our understanding of

this case has been aided by theoretical attempts to

deal with the effects of a small magnetic field on variable range hopping in doped semiconductors.

One of the recent developments

the study of a directed-hopping

in

this area has been

effect on the magnetoresistance

discuss some experimental evidence

for the

analogue of this

and later we effect

in

a

granular metal.

It

is

not surprising that the magnetoresistance

in

spectrum of