Modern Aspects of Electrochemistry
Recognized experts present incisive analysis of both fundamental and applied problems in this continuation of a highly acclaimed series. Topics discussed include: A review of the literature on the potential-of-zero charge by Trasatti and Lust. A thorough
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LIST OF CONTRIBUTORS RYOICHI AOGAKI
TORIBIO FERNANDEZ OTERO
National Research Laboratory for Magnetic Science Japan Science and Technology Corporation l-l-56 Shibashimo Kawaguchi, Saitama 333-0848 JAPAN
Facultad de Quimica Depto. de Quemica-Fisica Laboratorio de Electroquimica Pa Manual de Lardizabal s/n Apdo. De Correos 1072 20080 San Sebastian, Spain
GERALD L. BAUER 3M Chemicals 3M Center Blg. 236-3C-89 St. Paul, MN 55144-1000 W. VES CHILDS 3M Chemicals 3M Center Blg. 236-3C-89 St. Paul, MN 55144-1000 ENN LUST Department of Physical Chemistry and Electrochemistry University of Milan Laboratory of Electrochemistry Via Venezian, 21-20133 Milan, Italy
PETER G. PICKUP Department of Chemistry Memorial University of Newfoundland St. John’s, Newfoundland Canada A1B 3X7 SERGIO TRASATTI Department of Physical Chemistry and Electrochemistry University of Milan Laboratory of Electrochemistry Via Venezian, 21-20133 Milan, Italy H. TRIBUTSCH Hahn-Meitner-Institut Bereich Physikal. Chemie Glienicker Str. 100 D-14109 Berlin, Germany
MODERN ASPECTS OF ELECTROCHEMISTRY No. 33 Edited by
RALPH E. WHITE University of South Carolina
Columbia, South Carolina
J. O’M. BOCKRIS Texas A&M University
College Station, Texas
and
B. E. CONWAY University of Ottawa Ottawa, Ontario. Canada
KLUWER ACADEMIC PUBLISHERS NEW YORK, BOSTON, DORDRECHT, LONDON, MOSCOW
eBook ISBN: Print ISBN:
0-306-46917-0 0-306-45968-X
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Preface This volume contains six chapters and a cumulative index for numbers 1–33. The topics covered include the potential of zero charge; nonequilibrium fluctuation in the corrosion process; conducting polymers, electrochemistry, and biomimicking processes; microwave (photo)electrochemistry; improvements in fluorine generation; and electronically conducting polymer films. Chapter 1 is a review of literature on the potential of zero charge. Trasatti and Lust discuss the concept of potential of zero charge, electrode potentials, and energy scales, and the relation of the potential of zero charge to other quantities. The experimental aspects of zero charge unfold as they discuss methods for the measurement of the potential of zero charge, estimation of the surface area of solid electrodes, and experimental data. They analyze experimental data by discussing comparisons of compilations, crystal-face specificity, the potential of zero charge and work function, ultrahigh vacuum versus solution data, the concept of “hydrophilicity,” other solvents, and indirect evidence of the “interfacial parameter” scale. The second chapter is by Aogaki and includes a rev
