Modern Aspects of Electrochemistry
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LIST OF CONTRIBUTORS K.-P. CHARLE Fritz Haber Institute Max Planck Society D-I000 Berlin 33, West Germany HUKY. CHEH Department of Chemical Engineering and Applied Chemistry Columbia University New York, New York 10027 DRAGUTIN M. DRAZIC Faculty of Technology and Metallurgy University of Belgrade 11001 Belgrade, Yugoslavia E. I. KHRUSHCHEVA A. N. Frumkin Institute of Electrochemistry Academy of Sciences of the USSR 117071 Moscow, USSR M. D. MAKSIMOVIC Faculty of Technology and Metallurgy University of Belgrade 11001 Belgrade, Yugoslavia
ANTHONY M. PESCO AT&T Bell Laboratories Murray HilI, New Jersey 07974 PETER N. PINTAURO Department of Chemical Engineering Tulane University New Orleans, Louisiana 70118 K. I. POPOV Faculty of Technology and Metallurgy University of Belgrade 11001 Belgrade, Yugoslavia M. R. TARASEVICH A. N. Frumkin Institute of Electrochemistry Academy of Sciences of the USSR 117071 Moscow, USSR MARK W. VERBRUGGE Physical Chemistry Department General Motors Research Laboratories Warren, Michigan 48090-9055 F. WILLIG Fritz Haber Institute Max Planck Society D-lOOO Berlin 33, West Germany
MODERN ASPECTS OF ELECTROCHEMISTRY No. 19 Edited by
B.Department E.CONWAY of Chemistry University of Ottawa Ottawa, Ontario, Canada
J. Department O'M. BOCKRIS of Chemistry Texas A&M University College Station, Texas
and
RALPH E. WHITE
Department of Chemical Engineering Texas A&M University College Station, Texas
PLENUM PRESS • NEW YORK AND LONDON
The Library of Congress cataloged the first volume of this title as follows: Modern aspects of electrochemistry. no. [1] Washington, Butterworths, 1954v. illus., 23 cm. No. 1-2 issued as Modern aspects series of chemistry. Editors: no. 1J. Bockris (with B. E. Conway, No. 3Imprint varies: no. 1, New York, Academic Press. - No.2, London, Butterworths. 1. Electrochemistry-Collected works. I. Bockris, John O'M. ed. II. Conway, B. E. ed. (Series: Modern aspects series of chemistry) QD552.M6 54-12732 rev
ISBN 978-1-4684-8669-8 ISBN 978-1-4684--8667-4 (e8ook) DOl 10.1007/978-1-4684-8667-4
© 1989 Plenum Press, New York Softcover reprint of the hardcover 15t edition 1989 A Division of Plenum Publishing Corporation 233 Spring Street, New York, N.Y. 10013
All rights reserved No part of this book may be reproduced, stored in a retrieval system, or transmitted in any form or by any means, electronic, mechanical, photocopying, microfilming, recording, or otherwise, without written permission from the Publisher
Preface The present volume is comprised of six chapters covering topics having both fundamental and substantial applied significance in electrochemistry: ion-exchange membrane behavior, corrosion and metal deposition, semiconductor charge injection, and the electrocatalytic properties of carbon. In the first chapter, Verbrugge and Pintauro examine transport models for ion-exchange membranes using approaches from the direction of electrochemical thermodynamics of irreversible processes and others. The properties ofth~ models are examined quantitatively in some mathem
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