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I7.3.1

Organic - based Magnetic Thin Films by Low Temperature CVD Ruth Shima Edelstein,1 Jung-Woo Yoo,1 N. P. Raju,1 Jeremy D. Bergeson,1 Konstantin I. Pokhodnya1,2, Joel S. Miller,2 and Arthur J. Epstein1 1 Department of Physics and Department of Chemistry, The Ohio State University, Columbus, OH 43210-1117, U.S.A 2 Department of Chemistry, University of Utah, Salt Lake City, UT 84112-0850, U.S.A.

ABSTRACT We describe how the composition of an organic - based magnet can be controlled by varying the Chemical Vapor Deposition (CVD) conditions. A study was conducted for the Co2(CO)8 / TCNE system to form cobalt tetracyanoethylene [Co(TCNE)x, x~2, a paramagnetic material], and for the V(CO)6 / TCNEx system to form vanadium tetracyanoethylene [V(TCNE)x, x~2, a ferrimagnetic material]. Thin V(TCNE)x, x~2 films (~0.05-0.5 µm) with room temperature conductivity of 10-4

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